Experimental Study on Mineral Dissolution and Carbonation Efficiency Applied to pH-Swing Mineral Carbonation for Improved CO2 Sequestration
نویسندگان
چکیده
Mineral carbonation incurs high operating costs, as large amounts of chemicals and energy must be used in the process. Its implementation on an industrial scale requires reducing expenditures consumption. Thus, this work aimed to investigate significant factors involved pH-swing mineral their effects CO2 capture efficiency. A central composite rotatable design (CCRD) was employed for optimizing operational parameters acid dissolution serpentinite. The results showed that temperature exerts a effect magnesium dissolution. By adjusting reaction 100 °C setting hydrochloric concentration 2.5 molar, 96% extraction achieved within 120 min 91% 30 reaction. optimal efficiency carbon dioxide 40–50%, at higher values than those found literature, 90% 150 bar pressures. It it is technically possible reduce time maintain levels above through present experiments.
منابع مشابه
Sequestration of Martian CO2 by mineral carbonation
Carbonation is the water-mediated replacement of silicate minerals, such as olivine, by carbonate, and is commonplace in the Earth's crust. This reaction can remove significant quantities of CO2 from the atmosphere and store it over geological timescales. Here we present the first direct evidence for CO2 sequestration and storage on Mars by mineral carbonation. Electron beam imaging and analysi...
متن کاملCO2 mineral sequestration: physically activated dissolution of serpentine and pH swing process
The effect of the physical activation on the dissolution of serpentine was investigated and a pH swing scheme was developed to improve the overall conversion of the CO2 mineral sequestration process. Various methods of the surface agitation such as ultrasound, acoustic, and internal (in-situ) grinding were examined for their effectiveness in removing the diffusion limiting SiO2 layer in order t...
متن کاملA review of mineral carbonation technologies to sequester CO2.
Carbon dioxide (CO2) capture and sequestration includes a portfolio of technologies that can potentially sequester billions of tonnes of CO2 per year. Mineral carbonation (MC) is emerging as a potential CCS technology solution to sequester CO2 from smaller/medium emitters, where geological sequestration is not a viable option. In MC processes, CO2 is chemically reacted with calcium- and/or magn...
متن کاملCarbon Sequestration via Mineral Carbonation: Overview and Assessment
This report is being written for the Carbon Sequestration Initiative at the request of two members, GM and ChevronTexaco. The purpose is to give a brief overview and assessment of carbon sequestration by mineral carbonation (referred to as “mineral sequestration” in this report). The assessment is to highlight areas that need development in order for this technology to become commercial, not to...
متن کاملCarbon dioxide sequestration in cement kiln dust through mineral carbonation.
Carbon sequestration through the formation of carbonates is a potential means to reduce CO2 emissions. Alkaline industrial solid wastes typically have high mass fractions of reactive oxides that may not require preprocessing, making them an attractive source material for mineral carbonation The degree of mineral carbonation achievable in cement kiln dust (CKD) underambienttemperatures and press...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: Energies
سال: 2023
ISSN: ['1996-1073']
DOI: https://doi.org/10.3390/en16052449